Hi Jfkb2,
Sounds to me like your linkage may be sticking somewhere.
I've recently gone through some automatic transmission issues. The harsh shifting on the early SL's can break the slip joint / yoke in the differential. Ask me how I know this. The later 60's SL's got a beefier slip joint. So, avoid driving it until you can check it out.
My first thought is to thoroughly check all the linkage and ESPECIALLY THE SOLENOID on the the top of the transmission. It's not visible from under the car and often gets missed while lubing the linkage. The solenoid and linkage should be accessible through a small cover under the carpet, on the passengers side of the transmission tunnel very near where the passengers food would rest. This solenoid releases the hydraulic pressure while the car is coming to a stop. If the pressure is not released, the transmission will down shift very harshly, especially from 3rd to 2nd.
I'd check, clean and lube (a drop of ATF works great) all the linkage while your at it, but I wouldn't change any adjustments.
Just my 2 cents and it's a place to start. Good luck, hope it helps.
Ed Riefstahl
Erie, PA
1966 230SL (Ms Magoo)
1970 280S (Miss Daisy)
1989 300SE (Majestic)
1999 BMW Z3 5 speed
1991 BMW 318I 5 Speed
1997 Toyota Paseo Convertible - Red 5 speed (have you ever seen one?)
1997 Ford Ranger step side (Mater)
2023 Mazda CX 5